Abstract
Neutron and X-ray scattering experiments have provided mounting evidence for spin and charge ordering phenomena in underdoped cuprates. These range from early work on stripe correlations in Nd-LSCO to the latest discovery of charge-density-waves in YBa2Cu3O6 + x. Both phenomena are characterized by a pronounced dependence on doping, temperature and an externally applied magnetic field. Here, we show that these electron-lattice instabilities exhibit also a previously unrecognized bulk-surface dichotomy. Surface-sensitive electronic and structural probes uncover a temperature-dependent evolution of the CuO2 plane band dispersion and apparent Fermi pockets in underdoped Bi-2 Sr2-x La-x CuO6 + delta (Bi2201), which is directly associated with an hitherto-undetected strong temperature dependence of the incommensurate superstructure periodicity below 130 K. In stark contrast, the structural modulation revealed by bulk-sensitive probes is temperature-independent. These findings point to a surface-enhanced incipient charge-density-wave instability, driven by Fermi surface nesting. This discovery is of critical importance in the interpretation of single-particle spectroscopy data, and establishes the surface of cuprates and other complex oxides as a rich playground for the study of electronically soft phases.
Original language | English |
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Article number | 1977 |
Number of pages | 7 |
Journal | Nature Communications |
Volume | 4 |
DOIs | |
Publication status | Published - Jul-2013 |
Keywords
- HIGH-T-C
- HIGH-TEMPERATURE SUPERCONDUCTORS
- FERMI-SURFACE
- STRIPE ORDER
- CUPRATE SUPERCONDUCTORS
- PSEUDOGAP STATE
- CRYSTAL-STATE
- BI2SR2CACU2O8+DELTA
- PHASE
- CA2-XNAXCUO2CL2